Download Synthesis of Heterocycles via Multicomponent Reactions II by Géraldine Masson, Luc Neuville (auth.), Romano V. A. Orru, PDF

By Géraldine Masson, Luc Neuville (auth.), Romano V. A. Orru, Eelco Ruijter (eds.)

Géraldine Masson, Luc Neuville ∙ Carine Bughin ∙ Aude Fayol ∙ Jieping Zhu Multicomponent Syntheses of Macrocycles Thomas J.J. Müller Palladium-Copper Catalyzed Alkyne Activation as an access to Multicomponent Syntheses of Heterocycles Rachel Scheffelaar ∙ Eelco Ruijter ∙ Romano V.A. Orru Multicomponent response layout options: in the direction of Scaffold and Stereochemical variety Nicola Kielland ∙ Rodolfo Lavilla contemporary advancements in Reissert-Type Multicomponent Reactions Jitender B. Bariwal ∙ Jalpa C. Trivedi ∙ Erik V. Van der Eycken Microwave Irradiation and Multicomponent Reactions Irini Akritopoulou-Zanze ∙ Stevan W. Djuric purposes of MCR-Derived Heterocycles in Drug Discovery

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With respect to the relatively low molecular mass, these chromophores display a rather favorable molecular figures of merit, b0m/Mw, where Mw is the molar mass. , glass transitions, a favorable property for composites in photo refractive materials. Based upon the peculiar reactivity of nitrothienyl substituted alkynes a one-pot three-component coupling-aminovinylation sequence to push-pull chromophores was readily developed [43]. Terminal alkynes 4 and sufficiently electron-deficient heteroaryl halides 5 were transformed under Sonogashira conditions into the expected coupling products, which were subsequently reacted in a one-pot fashion with secondary amines 2 to furnish the push-pull systems 6 in good yields (Scheme 4).

1 Domino Synthesis of 2-Substituted Quinolines . . . . . . . . . . . . . . . . . . . 2 Domino Synthesis of Spiro-Benzofuranones and Spiro-Benzoindolones . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 76 9 Conclusion and Outlook . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 79 References . . . .

4 Pyrimidines by a Two-Step Sequence of Consecutive 3CR of (Hetero)Arenes, Oxalyl Chloride, Alkynes, and Cyclocondensation with Guanidinium Salts . . . . 5 Benzo[b][1,4]Diazepines by a Consecutive 3CR of Acid Chlorides, Alkynes, and Ortho-Phenylene Diamines . . . . . . . . . . . . . . . . . . . . . . 6 Benzo[b][1,5]Thiazepines by a Consecutive 3CR of Acid Chlorides, Alkynes, and Ortho-Amino Thiophenols . . . . . . . . . . . . . . . . . . .

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